signature=49a139e45aae48095ba948d9ce05c91d,Identification of column-integrated dominant aerosols usi...

该研究利用AERONET站点1999年至2007年的数据,区分了主导气溶胶类型,包括矿物尘、碳质气溶胶和二次无机离子等。气溶胶光学深度、单散射反照率、吸收安格斯特罗姆指数和细粒子分数等参数用于分类。结果显示,春季矿物尘和含碳矿物尘最为常见,冬季黑碳和有机碳因取暖需求而增多,夏季则以二次无机离子为主。气溶胶类型的识别在各个具有不同源特性的全球站点得到了验证,证实了这种方法的有效性。

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Abstract

Dominant aerosols were distinguished from level 2 inversion products for the Anmyon Aerosol Robotic Network (AERONET) site between 1999 and 2007. Secondary inorganic ions, black carbon (BC) and organic carbon (OC) were separated from fine mode aerosols, and mineral dust (MD), MD mixed with carbon, mixed coarse particles were separated from coarse mode aerosols. Four parameters (aerosol optical depth, single scattering albedo, absorption Angstrom exponent, and fine mode fraction) were used for this classification. Monthly variation of the occurrence rate of each aerosol type reveals that MD and MD mixed with carbon are frequent in spring. Although the fraction among dominant aerosols and occurrence rates of BC and OC tend to be high in cold season for heating, their contributions are variable but consistent due to various combustion sources. Secondary inorganic ions are most prevalent from June to August; the effective radius of these fine mode aerosols increases with water vapor content because of hygroscopic growth. To evaluate the validity of aerosol types identified, dominant aerosols at worldwide AERONET sites (Beijing, Mexico City, Goddard Space Flight Center, Mongu, Alta Floresta, Cape Verde), which have distinct source characteristics, were classified into the same aerosol types. The occurrence rate and fraction of the aerosol types at the selected sites confirm that the classification in this study is reasonable. However, mean optical properties of the aerosol types are generally influenced by the aerosol types with large fractions. The present work shows that the identification of dominant aerosols is effective even at a single site, provided that the archive of the data set is properly available.

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