Virtually Structured Illumination For Terahertz Super-Resolution Imaging
Virtually Structured Illumination For Terahertz Super-Resolution Imaging
super-resolution imaging
J AMES P. F LEMING 1, 2, * , L UCY A. D OWNES 2 , J OHN M. G IRKIN 1 AND
K EVIN J. W EATHERILL 2
1 Centrefor Advanced Instrumentation, Department of Physics, Durham University, South Road, Durham
DH1 3LE, United Kingdom
arXiv:2504.12092v1 [physics.optics] 16 Apr 2025
2 Quantum Light and Matter Group, Department of Physics, Durham University, South Road, Durham DH1
3LE, United Kingdom
* [email protected]
1. Introduction
Imaging in the THz band (0.3-3 THz) [1] has many applications ranging from security screening [2]
and non-destructive testing [3] to biomedical diagnostics [4]. These applications take advantage
of the favorable properties of the THz frequency range, such as its ability to penetrate common
non-conducting materials like wood, paper, and plastics [5]. Additionally, its non-ionizing nature
makes it a safer alternative to higher-frequency penetrating radiation, further broadening its
appeal across various domains.
THz imaging can broadly be categorized into two general schemes: single-point (SP) detection
and focal-plane array (FPA) detection. While SP detectors typically acquire images by raster-
scanning a target object, FPA detectors can capture images in a single shot using a 2D array
of sensors for parallel acquisition. Through the use of far-field aperture-based raster scanning
techniques, SP detectors can achieve sub-diffraction limited spatial resolution and, when combined
with time-domain spectroscopy (TDS), can produce images with hyperspectral information.
However, the raster-scanning process is inherently slow, making SP detection unsuitable for
applications requiring rapid image acquisition. In contrast, FPA detectors offer significantly faster
imaging speeds by capturing images in a single-shot. Recent advancements in room-temperature
FPAs have led to commercially available THz cameras with video-rate acquisition performance.
However, despite these advances, THz FPA detectors generally suffer from low sensitivity, high
noise, provide no spectral information, and ultimately are constrained by diffraction-limited
spatial resolution.
Techniques to overcome the diffraction limit have been investigated in optical microscopy
for many years. One example of such super-resolution techniques is Structured Illumination
Microscopy (SIM) [6, 7]. SIM involves illuminating a sample with a known spatial pattern to
allow the extraction of high-frequency spatial information. This technique can increase spatial
resolution of images by up to a factor of two above the diffraction limit [8]. One downside of
SIM is that it requires the acquisition of numerous images in order to collect sufficient spatial
information. Whilst this is not a major issue for optical imaging where sensors are fast and
have low noise, it is a more significant problem in the THz range and previous attempts of
super-resolution imaging at THz frequencies have either been purely through computational
enhancement [9, 10] or demonstrated via SP detection [11].
Recently, a novel THz FPA sensor based on THz-to-optical conversion in room temperature,
optically pumped atomic vapor has emerged [12, 13]. This technique has demonstrated very high
image acquisition rates in comparison to other room-temperature FPA sensors, and because images
are captured using standard optical cameras, sensors can be chosen to match the application.
Here, we make use of a fast atom-based THz imaging system to apply a variant of SIM
known as Virtually Structured Detection (VSD) [14, 15] to achieve THz super-resolution imaging.
Being able to perform super-resolution imaging at 0.55 THz holds promise for applications that
require high-speed and high-spatial resolution, while leveraging the deep penetrating properties
of 0.55 THz radiation.
𝑀˜ (k) = 𝛿 (k + p 𝜃 ) 𝑒 𝑖 𝜙 + 𝛿 (k − p 𝜃 ) 𝑒 −𝑖 𝜙 . (2)
Here, the modulation comprises of two delta functions, 𝛿 (k ± p 𝜃 ), which when convolved
˜
with the Fourier spectrum of the object, 𝑆(k), shifts the content of the spectrum by the spatial
frequency vector, ±p 𝜃 . This is a feature of the Fourier shifting property [20]. Under such
˜
modulation 𝑃(k), the Fourier transform of 𝑝(r), is realized as
˜ = 𝐻˜ (k) 𝑆(k ˜ − p 𝜃 )𝑒 −𝑖 𝜙 .
˜ + p 𝜃 )𝑒 𝑖 𝜙 + 𝑆(k
𝑃(k) (3)
These shifted Fourier bands 𝑆(k ˜ ± p 𝜃 ) contain higher spatial frequency information that
otherwise would be cut-off by the optical transfer function (OTF) of the imaging system
˜ ± p 𝜃 ) by changing the
𝐻˜ (k) = 𝐻˜ 𝑖𝑙 (k) 𝐻˜ 𝑑𝑒 (k). Solving Eq. (3) for the shifted Fourier bands 𝑆(k
phase of the modulation, 𝜙, allows for retrieval of the two shifted bands,
˜ ± p 𝜃 ) = 𝑃(k,
𝐻˜ (k) 𝑆(k ˜ 𝜙 = 0) ± 𝑖 𝑃(k,
˜ 𝜙 = 𝜋/2) . (4)
As the modulation is applied computationally, no additional image scans are required for the
additional phase. Unlike SIM, the reconstruction is phase artifact-free as the phase is exactly
defined [19]. Typically, attenuation of spatial frequencies caused by 𝐻˜ (k) can be restored via a
final deconvolution step
˜ ± p 𝜃 ) = deconvolve 𝑃(k,
˜ 𝜙 = 0) ± 𝑖 𝑃(k,
˜ 𝜙 = 𝜋/2) .
𝑆(k (5)
For this work, we opted not to deconvolve our images to assess the standalone performance of
the VSD technique. We direct the reader to the extensive use of various deconvolution algorithms
in the literature [21–24].
Super-resolution image reconstruction concludes by summation of the two shifted Fourier
bands, improving the spatial frequency extent for a theoretical maximum two-fold resolution
when |p 𝜃 | = kcutoff , the cut-off spatial frequency of the widefield system [25]. Such improvement
is observed across the scan-axis only. For near-isotropic resolution improvement, the angle over
which the sample is scanned is varied, typically as 𝜃 = 0°, 60° and 120°.
3. Experimental Implementation
Fig. 1. a) Energy ladder scheme in Cesium used for the conversion of 0.55 THz to
the green 535 nm via decay fluorescence. b) True-color composite image of the vapor
cell with 1 cm2 sensing area, both unfiltered background fluorescence and green signal
fluorescence are shown. c) Processed monochromatic THz image from the acquired
fluorescence signal.
Widefield THz images were collected using our atom-based imaging system, full details
of which are available in previous publications [13, 26]. To summarize, using infrared lasers,
frequency stabilized to atomic references [27, 28], we can promote alkali metals to highly excited
states, known as Rydberg states [29]. Rydberg states feature electric-dipole transitions that fall
within the THz frequency band and are therefore sensitive to resonant THz fields. Rydberg
states also spontaneously decay via probabilistic decay pathways back to the atomic ground state,
producing an optical fluorescence spectra. By illuminating a thermal vapor of optically pumped
alkali metal atoms with a resonant THz-field, the appropriate Rydberg transition can be driven,
which will then decay to produce a detectable optical fluorescence signal. By shaping each laser
with a combination of cylindrical lenses, overlapping lightsheets can be formed, constructing an
active sensing focal-plane. High-speed, high-sensitivity focal-plane THz imaging is therefore
realized by efficient THz-to-optical conversion. The sub-microsecond decay rates of the Rydberg
states allows theoretical imaging rates in the 1 MHz range. In practice the imaging frame-rate
is limited by the signal-to-noise and available throughput of the optical readout system, which
has been demonstrated to a maximum of 12,000 frames per second, an almost three-orders of
magnitude improvement when compared to the state-of-the-art commercial THz cameras [26].
In this study, we operate our Rydberg-based THz imaging system at 0.55 THz by using the
14P3/2 → 13D5/2 transition in Cesium, as shown in Fig. 1a. A Cesium thermal vapor (Fig. 1b)
is contained in a heated quartz cell and maintained at 45◦ , which maximizes the fluorescence
THz Sensi�ve
Op�cal
Imaging Lens Atom Imager
Readout
Object mask
Lens relay
Line mask
f Linescan
Images
f
Phase
f Images
f
Collimated THz
Beam Input
vs. Digital modula�on
+ stacking
Fourier
Widefield Super-resolved reconstruc�on
Image Image
signal without the thermal vapor becoming optically thick to the infrared excitation lasers. The
vapor cell provides optical access on all four sides. Three frequency-stablized infrared lasers
(𝜆 = 852 nm, 1470 nm, 843 nm) drive the three-step excitation scheme and prepare Cesium in
the 14P3/2 state. The size of the vapor cell and available laser power produces an active sensing
region of 1 cm2 . Narrow-band, resonant 550 GHz continuous-wave THz illumination is provided
by a Virginia Diodes Inc. amplifier multiplier chain (AMC). A stable microwave generator seeds
the AMC, and the frequency is upconverted by a factor of 36, providing a maximum power output
of 5 mW. A power output of 0.3 mW was used to illuminate the target without saturating the
imaging system.
To implement VSD, the required line-profile illumination was generated via a mask with a
sub-diffraction, 250 𝜇m wide slit. The illuminated mask was then imaged onto the object plane
using an image relay of two aspheric PTFE plano-convex lenses (d = 50.8 mm, f = 75 mm),
as shown in Fig. 2. The mask was mounted on a manual rotation stage in order to set the scan
angle 𝜃. Unlike previous optical implementations [14, 15, 19], the scanning process occurs by
translating the object normal to the fixed line illumination, using a pair of translation stages
(Thorlabs MTS50-Z8). A transmissive mask was used as the object of interest to image, placed
at the output plane of the image relay. Both illumination and object masks were produced by
milling copper-clad FR4 board. A common material used in electronic circuit board production,
the copper foil cladding blocks transmission, while FR4 substrate is transmissive at 0.55 THz.
Widefield full-frame images of the object are taken using our atomic THz imager. A commercial
1x silicon objective lens (i2S, d = 60 mm, f = 70 mm) images onto the THz-sensitive atomic
vapor. The optical fluorescence from the vapor was captured by an Andor iXon Ultra 888
EMCCD camera, under a 200 ms exposure. An appropriate bandpass filter was used to isolate
the signal from superfluous background fluorescence. Images are post-processed by subtracting
a background frame to further isolate the signal [26]. Each captured image was then cropped
to a region of interest (ROI) around the line-center of the illumination. A ROI with width of
the expected Airy disc size was found to be an adequate trade-off between signal-to-noise and
rejection of unwanted diffracted illumination. To generate comparative true widefield images, the
illumination mask was removed and the object mask centered to produce an equivalent uniformly
illuminated, single-shot widefield image.
4. Results
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