The Effect of Microstructural Morphology
The Effect of Microstructural Morphology
a r t i c l e i n f o a b s t r a c t
Article history: Micromechanical models with idealized and simplified shapes of inhomogeneities have been widely
Received 22 November 2013 used to obtain the average (macroscopic) mechanical response of different composite materials. The
Accepted 10 February 2014 main purpose of this study is to examine whether the composites with irregular shapes of inhomo-
Available online 20 February 2014
geneities, such as in the aluminum–alumina (Al–Al2 O3 ) composites, can be approximated by considering
idealized and simplified shapes of inhomogeneities in determining their overall macroscopic mechani-
Keywords:
cal responses. We study the effects of microstructural characteristics, on mechanical behavior (elastic,
Aluminum–alumina composites
inelastic, and degradation) of the constituents, and shapes and distributions of the pores and inclu-
Micro-structures
Elastic
sions (inhomogeneities), and thermal stresses on the overall mechanical properties and response of the
Inelastic Al–Al2 O3 composites. Microstructures of a composite with 20% alumina volume content are constructed
Thermal stress from the microstructural images of the composite obtained by scanning electron microscopy (SEM). The
SEM images of the composite are converted to finite element (FE) meshes, which are used to determine
the overall mechanical response of the Al–Al2 O3 composite. We also construct micromechanics model
by considering circular shapes of the inhomogeneities, while maintaining the same volume contents
and locations of the inhomogeneities as the ones in the micromechanics model with actual shapes of
inhomogeneities. The macroscopic elastic and inelastic responses and stress fields in the constituents
from the micromechanics models with actual and circular shapes of inhomogeneities are compared and
discussed.
© 2014 Elsevier Ltd. All rights reserved.
http://dx.doi.org/10.1016/j.mechrescom.2014.02.003
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50 P. Gudlur et al. / Mechanics Research Communications 57 (2014) 49–56
Fig. 2. FE meshed model #3 of A-20 composite sample with (a) actual shape and (b) circular shape of reinforcement and pores; stress ( 11 ) contour for (c) actual shape and
(d) circular shape of reinforcement and pores due to thermal stress.
overall/effective responses of the composites. We then study the aluminum follows the deformation theory of plasticity (Hencky–
effect of idealizing the shapes of the inclusions (particles and pores) Ilyushin):
on the effective response of the composites. Using the image anal-
ysis software ImageJ, the area of the actual shaped reinforcements p Sij kk
and pores are calculated along with their centroids (see Gudlur, εij = εeij + εij + εth ; εeij = + ı ; εth = ˛ıij (T − Tref )
ij 2G 9K ij ij
2013), for each of the FE meshed models of the A-20 sample ⎧
shown in Fig. 1b. Using ABAQUS Python script, circular shaped ⎨ 3 ¯ Sij , F = 0 (2)
p
εij = 2 ¯
reinforcements and pores, with the areas same as those of their
⎩
corresponding actual shaped reinforcement and pores, are substi- 0, F<0
tuted in their places at their respective centroids. Fig. 2(a and b)
illustrates the FE mesh 3 with actual and circular inhomogeneities.
p p p
Next, we used the micromechanics models to study the inelastic The equivalent plastic strain is ¯ = (2/3)εij εij , where εij is
deformation and degradation behaviors in the composites, incor- the
component of the plastic strain, and the effective stress is ¯ =
porating the thermal stress effect. The alumina is modeled as linear (3/2)Sij Sij . It is assumed that the material is rate-independent
elastic while the aluminum is assumed to exhibit an elastic–plastic p
and the yield criterion is given as F = ¯ − y (εij ). The aim of this
deformation. Both aluminum and alumina are modeled as isotropic
study is to examine the effect of microstructures, i.e., porosity, local
materials undergoing small deformation gradients. The linear elas-
yielding, thermal stress, distribution of the alumina particles in the
tic constitutive model for the alumina is:
homogeneous aluminum matrix, and shapes of inhomogeneities,
on the overall linear elastic moduli2 and response of the Al–Al2 O3
Sij kk composites. It is noted that due to the plane stress assumption the
εij = εeij + εth = + ı + ˛ıij (T − Tref ) (1) out of plane strain component arises from imposing zero out of
ij 2G 9K ij
plane stress condition.
Model E (GPa)
The FE simulation is carried out in two steps. The first step is pre-
scribing a uniform temperature change from 200 ◦ C, which is con- FE-1 83.28 0.313
sidered as the stress-free temperature3 based on our previous work, FE-2 86.67 0.311
FE-3 83.70 0.314
Gudlur et al. (2014), to 25 ◦ C and examining the residual (remain- FE-4 88.05 0.315
ing thermal) stresses. The thermal expansion coefficients for the Mori–Tanaka 87.00 0.330
aluminum and alumina at room temperature are 28 × 10−6 /◦ C and
4.6 × 10−6 /◦ C, respectively. The second step is simulating a uni-
axial mechanical boundary condition to determine the uniaxial The uniaxial compressive stress is simulated by prescribing a
elastic moduli and stress–strain response of the composite. The uniaxial displacement ı0 = 2.5 × 10−3 mm, which corresponds to
elastic moduli of the aluminum and alumina at room tempera- the axial strain 5%4 followed by removal of the strain.
ture are 65 GPa and 370 GPa, respectively. The Poisson’s ratios of
the aluminum and alumina are 0.35 and 0.22, respectively. The 3.1. Linear elastic properties
above thermal expansion and elastic properties of the aluminum
are obtained from Gudlur et al. (2012). The stress–strain response of The linear responses from the FE analyses are first studied and
the aluminum obtained from literature Moosbrugger (2002) is used compared to the ones obtained from the experiment from the
to model the plastic deformation of aluminum in the numerical nondestructive testing, resonant ultrasound spectroscopy (RUS).
analyses and the yield stress of aluminum is taken as 33 MPa. Table 1 presents the values of Elastic moduli and Poisson’s ratios
Consider a FE microstructure of a square region with a side from the six FE meshes considered. The first four FE meshes (FE-
length L placed in the 2D Cartesian coordinate system with the 1, FE-2, FE-3, and FE-4) have 50 m × 50 m square region, while
bottom left corner of the microstructure is at the origin. The FE-5 and FE-5 have 100 m × 100 m square region. We first per-
microstructure is subjected to the following displacement bound- formed a convergence study in terms of number of elements (mesh
ary conditions: sizes) used in the FE analyses for the first four FE meshes, as shown
in Table 1. The average size of the element in the FE analyses
u1 (0, x2 ) = u2 (x1 , L) = 0.0, u1 (L, x2 ) = C and u2 (x1 , 0) = ıo (4) with coarse elements is 3.27 × 10−4 mm × 3.27 × 10−4 mm, while
the one with finer elements is 1.96 × 10−4 mm × 1.96 × 10−4 mm. In
where u1 and u2 are the displacements in the x1 - and x2 -directions, the above FE analyses the effect of thermal stresses on the effective
respectively. The linear elastic modulus is determined by prescrib- elastic moduli and Poisson’s ratios of composites is also considered
ing a relatively small uniaxial compressive stress ¯ 22 (x1 , 0) = 0 = by prescribing a uniform temperature change from 200 ◦ C to 25 ◦ C
1 MPa and monitoring the corresponding overall (average) strain prior to determining the elastic properties. We concluded that the
ε̄22 . By prescribing a relatively small stress we can minimize effects coarse elements are capable in capturing the overall properties of
of the possible plastic deformation due to mechanical loading. The the composites while significantly reduce the computational cost.
corresponding transverse displacement along the boundary of the The rest of the FE analyses are performed using coarse elements.
microstructure is constrained to be uniform. The effective elastic It is also seen that the smaller RVE size is capable in represent-
modulus Ē and Poisson effect ¯ are defined as: ing the heterogeneities in composites. For comparison, we also
determined the overall elastic properties of composites without
ı0 ¯ 22
ε̄22 = ; Ē = considering the thermal (residual) stress effect. Table 2 lists the
L ε̄22
(5) effective elastic modulus and Poisson’s ratios from four FE meshes
C ¯ 22 and from Mori–Tanaka micromechanics model. It is seen that the
ε̄11 = ; =-
L ε̄22 elastic moduli without the residual stress effect are about 12 GPa
higher than the ones with the residual stress effect. It is also noted
that the effective elastic properties from the four FE analyses are
3
The composite processing involves curing at 600 ◦ C followed by slow cooling closed to the ones of Mori–Tanaka model with 20% alumina volume
down to room temperature (about 7 h). During the cooling process, the aluminum contents, in which an idealized microstructure of a composite with
experiences stress relaxation at elevated temperatures which reduces the pre- a solid sphere embedded in homogeneous matrix is considered.
stresses in the constituents due to the previous processing conditions. It might not
be possible to eliminate the entire pre-stress by the stress-relaxation; however
we consider the temperature at which the pre-stress is minimum as our zero-
4
stress temperature. Further continuing the cooling process to room temperature This is an engineering strain defined as the overall axial displacement divided
will eventually increase the residual-stresses. by the original length of the specimen.
P. Gudlur et al. / Mechanics Research Communications 57 (2014) 49–56 53
80 with actual parƟcle shape In the microstructure with actual shapes of inhomogeneities, the
with circular parƟcles maximum tensile stress is around 300 MPa, while the maximum
ElasƟc Modulus (GPa)
Fig. 4. The effect of shapes of inhomogeneities on the overall inelastic response of composites under uniaxial compression.
54 P. Gudlur et al. / Mechanics Research Communications 57 (2014) 49–56
Fig. 5. Stress contour in the transverse direction ( 11 ) of FE meshed model #3 at maximum applied strain (ε22 = 5%). Left: actual shapes of inhomogeneities and right: circular
shapes of inhomogeneities.
Fig. 6. Uniaxial tensile response of composites with inelastic and degradation behaviors for (a) FE-1 and (b) FE-3.
fields due to the effect of stress concentration. In this study, the dis- stress and degradation fields in FE meshed model #1. As seen in
tribution of stress fields in the composite models with actual and the figures, the composite with actual shapes of inhomogeneities
circular microstructures only slightly influences the macroscopic shows stress and degradation fields with higher magnitude as com-
inelastic response of the composites. pared to the composite with circular shapes of inhomogeneities,
We now consider the possibility of degradation in the brittle especially in the brittle inclusions. The degrading elastic properties
inclusions due to existence of tensile stresses. For this purpose, of the inclusions do not have significant effect in this composite sys-
we define the degradation parameter, according to Eq. (3) and tem, as the response is dominated by the ductile matrix behaviors.
the elastic modulus of the alumina decrease with the degradation This might also be because of the relatively low content of the brittle
E = E0 (1 − d), where E0 is the elastic modulus of alumina in absence alumina (20%). It is noted that sharp edges of the inhomogeneities
of degradation. It is assumed that degradation occurs when the in the microstructures with actual shapes of inhomogeneities lead
normal stresses in the alumina are under tension. The following to high localized stresses (see contours in Figs. 2, 5 and 7). In real-
function is considered to numerically study the effect of degrada- ity, high localized tensile stresses would cause cracks to initiate and
tion: propagate in the composite bodies. When the effect of cracking in
the composite on the overall macroscopic mechanical performance
f (εij ) = ˛ ε211 + ε222 + ε233 ; ε11 > 0, or ε22 > 0, or ε33 > 0 of the composites is considered, perhaps it is necessary to consider
composites with actual shapes of inhomogeneities (see Williams
(6) et al., 2012).
Fig. 7. Transverse stress and degradation contours from FE meshed model #1 with actual (top) and idealized (bottom) inhomogeneities.
alumina and inelastic response of the aluminum matrix. Further- materials. The effect of degradation in the brittle alumina under
more, the effect of the degradation in the brittle alumina due tension was also investigated. Once again, it was observed that the
to tensile stresses/strains, which reduces the elastic modulus of composites with actual shapes of inhomogeneities experience
the alumina, on the overall stress–strain response of the com- higher magnitude of stress and degradation fields as compared to
posite was examined. Two composite microstructures with actual the ones with circular shapes of inhomogeneities. However, the
and idealized shapes of the inhomogeneities were considered. The macroscopic stress–strain responses from the two composites are
stress fields in the two microstructures due to prescribed thermal very close, which shows the insignificant overall effect of the shapes
and mechanical stimuli were compared and their effects on the of inhomogeneities on the macroscopic mechanical responses. The
overall macroscopic mechanical response of the composites were reason might be due to a relatively low volume content of inhomo-
examined. Micromechanics models with idealized and simplified geneities (around 20% volume contents of the composites), in which
shapes of inhomogeneities have been widely used to obtain the the macroscopic response is dominated by the matrix behavior. It is
average (macroscopic) response of composites due to their rela- also noted that this study does not consider fracture in the compos-
tively low costs in providing analytical and numerical solutions. ites due to severe stresses localized in the constituents that might
The main purpose of this study is to examine whether the com- lead to crack initiation and propagation.
posites with irregular shapes of inhomogeneities, such as in the
Al–Al2 O3 composites, can be approximated by considering ideal-
Acknowledgements
ized and simplified shapes of inhomogeneities in determining their
overall macroscopic mechanical responses.
This research is sponsored by the National Science Foundation,
We found that the linear elastic modulus of the Al–Al2 O3 com-
under the grant CMMI-1030836 and Air Force Office of Scientific
posite, ignoring the effect of thermal stresses, can be well predicted
Research AFOSR FA 9550-10-1-0002.
by the Mori–Tanaka model with a solid spherical alumina inclusion.
We also found that the linear elastic properties of composites with
actual and circular inhomogeneities are very close. This shows the References
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